Optical Production of Stable Ultracold 88^{88}Sr2_2 Molecules

preprint2012arXivOpen access

Abstract

We have produced large samples of ultracold 88^{88}Sr2_2 molecules in the electronic ground state in an optical lattice. The molecules are bound by 0.05 cm−1^{-1} and are stable for several milliseconds. The fast, all-optical method of molecule creation via intercombination line photoassociation relies on a near-unity Franck-Condon factor. The detection uses a weakly bound vibrational level corresponding to a very large dimer. This is the first of two steps needed to create Sr2_2 in the absolute ground quantum state. Lattice-trapped Sr2_2 is of interest to frequency metrology and ultracold chemistry.

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