Manipulating shear-induced non-equilibrium transitions by feedback control

preprint2014arXivOpen access

Abstract

Using Brownian Dynamics (BD) simulations we investigate non-equilibrium transitions of sheared colloidal films under controlled shear stress σxzσ_{\mathrm{xz}}. In our approach the shear rate γ˙\dotγ is a dynamical variable, which relaxes on a timescale τcτ_c such that the instantaneous, configuration-dependent stress σxz(t)σ_{\mathrm{xz}}(t) approaches a pre-imposed value. Investigating the dynamics under this "feedback-control" scheme we find unique behavior in regions where the flow curve σxz(γ˙)σ_{\mathrm{xz}}(\dotγ) of the uncontrolled system is monotonic. However, in non-monotonic regions our method allows to {\em select} between dynamical states characterized by different in-plane structure and viscosities. Indeed, the final state strongly depends on τcτ_c relative to an {\em intrinsic} relaxation time of the uncontrolled system. The critical values of τcτ_c are estimated on the basis of a simple model.

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