Abstract

Neutron scattering techniques are used to investigate the crystalline and magnetic structure of LuFe0.75_{0.75}Mn0.25_{0.25}O3_{3} in bulk polycrystalline form. We find that the crystalline structure is described by the hexagonal P63_{3}cm space group similar to that of thin-film LuFeO3_{3}, and that the system orders antiferromagnetically below TN_{N} = 134 K. Inelastic neutron scattering reveals nearest-neighbor superexchange parameters that are enhanced relative to LuMnO3_{3}. The observation of significant diffuse scattering above TN_{N} demonstrates the frustrated nature of the system; comparisons with similar materials suggest the ground state magnetic configuration is sensitive to local crystallographic distortions.

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