Magnetic anisotropy and entropy change in trigonal Cr0.62_{0.62}Te

preprint2019arXivOpen access

Abstract

We present a comprehensive investigation on anisotropic magnetic and magnetocaloric properties of the quasi-two-dimensional weak itinerant ferromagnet trigonal Cr0.62_{0.62}Te single crystals. Magnetic-anisotropy-induced satellite transition T∗T^* is observed at low fields applied parallel to the abab plane below TcT_c. The T∗T^* is featured by an anomalous magnetization downturn, similar to that in structurally related CrI3_3, and shows a monotonous shift towards lower temperature with increasing field. Magnetocrystalline anisotropy is also reflected in magnetic entropy change ΔSM(T,H)ΔS_M(T,H) and relative cooling power RCP. Given the high TcT_c, Cr0.62_{0.62}Te crystals are materials of interest for nanofabrication in basic science and applied technology.

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