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Low temperature studies of the excited-state structure of Nitrogen-Vacancy color centers in diamond

We report a study of the 3E excited-state structure of single nitrogen-vacancy (NV) defects in diamond, combining resonant excitation at cryogenic temperatures and optically detected magnetic resonance. A theoretical model of the excited-state structure is developed and shows excellent agreement with experimental observations. Besides, we show that the two orbital branches associated with the 3E excited-state are averaged when operating at room temperature. This study leads to an improved physical understanding of the NV defect electronic structure, which is invaluable for the development of diamond-based quantum information processing.

preprint2009arXivOpen access
A. BatalovV. JacquesF. KaiserP. SiyushevP. NeumannL. J. RogersR. L. McMurtrieN. B. MansonF. JelezkoJ. Wrachtrup
quant-ph
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Open access10 authors1 topic
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A. BatalovV. JacquesF. KaiserP. SiyushevP. NeumannL. J. RogersR. L. McMurtrieN. B. MansonF. JelezkoJ. Wrachtrup

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