Long coherence time of spin qubits in 12^{12}C enriched polycrystalline CVD diamond

preprint2012arXivOpen access

Abstract

Single defects in diamond and especially negatively charged nitrogen vacancy (NV) centers are very promising quantum systems with wide applications in physics and biology. It was shown that their coherence properties can be strongly improved by growing ultrapure diamond with low concentration of parasitic spins associated with nitrogen electron spins and nuclear spins related to 13^{13}C carbon isotope. Here we report a high quality 12^{12}C-enriched polycrystalline CVD diamond material with properties comparable with single crystals. We find single NVs in the grains of this material, which show extremely long electron spin coherence time T2>2 msT_2 > 2\,ms.

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