Intrinsic upper bound on two-qubit polarization entanglement predetermined by pump polarization correlations in parametric down-conversion

We study how one-particle correlations transfer to manifest as two-particle correlations in the context of parametric down-conversion (PDC), a process in which a pump photon is annihilated to produce two entangled photons. We work in the polarization degree of freedom and show that for any two-qubit generation process that is both trace-preserving and entropy-nondecreasing, the concurrence $C(ρ)$ of the generated two-qubit state $ρ$ follows an intrinsic upper bound with $C(ρ)\leq (1+P)/2$, where $P$ is the degree of polarization of the pump photon. We also find that for the class of two qubit states that is restricted to have only two non-zero diagonal elements such that the effective dimensionality of the two-qubit state is same as the dimensionality of the pump polarization state, the upper bound on concurrence is the degree of polarization itself, that is, $C(ρ)\leq P$. Our work shows that the maximum manifestation of two-particle correlations as entanglement is dictated by one-particle correlations. The formalism developed in this work can be extended to include multi-particle systems and can thus have important implications towards deducing the upper bounds on multi-particle entanglement, for which no universally accepted measure exists.

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