Interplay of the spin density wave and a possible Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5\mathrm{CeCoIn_5} in rotating magnetic field

preprint2020arXivOpen access

Abstract

The dd-wave superconductor CeCoIn5\mathrm{CeCoIn_5} has been proposed as a strong candidate for supporting the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state near the low-temperature boundary of its upper critical field. Neutron diffraction, however, finds spin-density-wave (SDW) order in this part of the phase diagram for field in the aa-bb plane, and evidence for the SDW disappears as the applied field is rotated toward the tetragonal cc axis. It is important to understand the interplay between the SDW and a possible FFLO state in CeCoIn5\mathrm{CeCoIn_5}, as the mere existence of an SDW does not necessary exclude an FFLO state. Here, based on a model constructed on the basis of available experiments, we show that an FFLO state competes with an SDW phase. The SDW state in CeCoIn5\mathrm{CeCoIn_5} is stabilized when the field is directed close to the aa-bb plane. When the field is rotated toward the cc axis, the FFLO state emerges, and the SDW phase disappears. In the FFLO state, the nodal planes with extra quasiparticles (where the superconducting order parameter is zero) are perpendicular to the field, and in the SDW phase, the quasiparticle density of states is reduced. We test this model prediction by measuring heat transported by normal quasiparticles in the superconducting state. As a function of field, we observe a reduction of thermal conductivity for field close to the aa-bb plane and an enhancement of thermal conductivity when field is close to the cc axis, consistent with theoretical expectations. Our modeling and experiments, therefore, indicate the existence of the FFLO state when field is parallel to the cc axis.

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