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Hydrogen-bond equilibria and life times in a supercooled monohydroxy alcohol

Dielectric loss spectra covering 13 decades in frequency were collected for 2-ethyl-1-hexanol, a monohydroxy alcohol that exhibits a prominent Debye-like relaxation, typical for several classes of hydrogen-bonded liquids. The thermal variation of the dielectric absorption amplitude agrees well with that of the hydrogen-bond equilibrium population, experimentally mapped out using near infrared (NIR) and nuclear magnetic resonance (NMR) measurements. Despite this agreement, temperature-jump NIR spectroscopy reveals that the hydrogen-bond switching rate does not define the frequency position of the prominent absorption peak. This contrasts with widespread notions and models based thereon, but is consistent with a recent approach.

preprint2011arXivOpen access
C. GainaruS. KastnerF. MayrP. LunkenheimerS. SchildmannH. J. WeberW. HillerA. LoidlR. Böhmer
cond-mat.soft
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Open access9 authors1 topic
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C. GainaruS. KastnerF. MayrP. LunkenheimerS. SchildmannH. J. WeberW. HillerA. LoidlR. Böhmer

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