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Hohenberg-Kohn theorem for the lowest-energy resonance of unbound systems

We show that under well-defined conditions the Hohenberg-Kohn theorem (HKT) can be extended to the lowest-energy resonance of unbound systems. Using the Gel'fand Levitan theorem, the extended version of the HKT can also be applied to systems that support a finite number of bound states. The extended version of the HKT provides an adequate framework to carry out DFT calculations of negative electron affinities.

preprint2006arXivOpen access
Adam WassermanNimrod Moiseyev
cond-mat.other
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Adam WassermanNimrod Moiseyev

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