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Field-Driven Self-Assembly of Magnetite Nanoparticles Investigated Using Small-Angle Neutron Scattering

The magnetic-field-induced assembly of magnetic nanoparticles (NPs) provides a unique and flexible strategy in the design and the fabrication of functional nanostructures and devices. We have investigated the field-driven self-assembly of core-shell magnetite NPs dispersed in toluene by means of in situ small angle neutron scattering (SANS). The form factor of the core-shell NPs was characterized and analyzed using SANS with polarized neutrons. Large-scale aggregation of magnetite NPs has formed above 0.02 T as indicated by very-small angle neutron scattering measurements. Three-dimensional long-range ordered superlattice of magnetite NPs was revealed under the application of moderate magnetic field. The crystal structure of the superlattice has been identified as a face-centered cubic one.

preprint2016arXivOpen access
Zhendong FuYinguo XiaoArtem FeoktystovVitaliy PipichMarie-Sousai AppavouYixi SuErxi FengW. T. JinThomas Brueckel
cond-mat.mes-hall
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Open access9 authors1 topic
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Zhendong FuYinguo XiaoArtem FeoktystovVitaliy PipichMarie-Sousai AppavouYixi SuErxi FengW. T. JinThomas Brueckel

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