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Excitons and carriers in transient absorption and time-resolved ARPES spectroscopy: an abinitio approach

I present a fully abinitio scheme to model transient spectroscopy signals in presence of strongly bound excitons. Using LiF as a prototype material, I show that the scheme is able to capture the exciton signature both in time-resolved ARPES and transient absorption experiments. The approach is completely general and can become the reference scheme for modelling pump and probe experiment in a wide range of materials.

preprint2022arXivOpen access
D. Sangalli
cond-mat.mtrl-sci
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D. Sangalli

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