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Paper detail

Exchange Interactions in a Dinuclear Manganese (II) Complex with Cyanopyridine-N-oxide Bridging Ligands

The structure and magnetic properties of oligonuclear manganese complex [Mn(hfa)2cpo]2 (where hfa is hexafluoroacetylacetonate dehydrate and cpo is 4-cyanopyridine-N-oxide) are presented. In the unit cell, the dinuclear molecules are well isolated from each other. The non-monotonous dependence of magnetic susceptibility is explained in terms of the hierarchy of exchange parameters by using exact diagonalization. The thermodynamic behavior of pure cpo and [Mn(hfa)2(cpo)]2 is simulated numerically in a dimer approximation by an extrapolation to spin S = 5/2. The Mn-Mn exchange integral is evaluated.

preprint2013arXivOpen access
A. S. MarkosyanI. Yu. GaidukovaA. V. RuchkinA. O. AnokhinV. Yu. IrkhinM. V. RyazanovN. P. Kuz'minaV. N. Nikiforov
cond-mat.mtrl-sci
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A. S. MarkosyanI. Yu. GaidukovaA. V. RuchkinA. O. AnokhinV. Yu. IrkhinM. V. RyazanovN. P. Kuz'minaV. N. Nikiforov

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