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Paper detail

Estimating Franck-Condon factors using an NMR quantum processor

Interaction of molecules with light may lead to electronic transitions and simultaneous vibrational excitations. Franck-Condon factors (FCFs) play an important role in quantifying the intensities of such vibronic transitions occurring during molecular photo-excitations. In this article, we describe a general method for estimating FCFs using a quantum information processor. The method involves the application of a translation operator followed by the measurement of certain projections. We also illustrate the method by experimentally estimating FCFs with the help of a three-qubit NMR quantum information processor. We describe two methods for the measurement of projections - (i) using diagonal tomography and (ii) using Moussa protocol. The experimental results agree fairly well with the theory.

preprint2014arXivOpen access
Sharad JoshiAbhishek ShuklaHemant KatiyarAnirban HazraT. S. Mahesh
quant-ph
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Sharad JoshiAbhishek ShuklaHemant KatiyarAnirban HazraT. S. Mahesh

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