Elusive Dzyaloshinskii-Moriya interaction in Fe3_3GeTe2_2 monolayer

preprint2020arXivOpen access

Abstract

Using symmetry analysis and density functional theory calculations, we uncover the nature of Dzyaloshinskii-Moriya interaction in Fe3_3GeTe2_2 monolayer. We show that while such an interaction might result in small distortion of the magnetic texture on the short range, on the longrange Dzyaloshinskii-Moriya interaction favors in-plane Néel spin-spirals along equivalent directions of the crystal structure. Whereas our results show that the observed Néel skyrmions cannot be explained by the Dzyaloshinskii-Moriya interaction at the monolayer level, they suggest that canted magnetic texture shall arise at the boundary of Fe3_3GeTe2_2 nanoflakes or nanoribbons and, most interestingly, that homochiral planar magnetic textures could be stabilized.

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