Electronic excitations and electron-phonon coupling in bulk graphite through Raman scattering in high magnetic fields

preprint2011arXivOpen access

Abstract

We use polarized magneto-Raman scattering to study purely electronic excitations and the electron-phonon coupling in bulk graphite. At a temperature of 4.2 K and in magnetic fields up to 28 T we observe KK-point electronic excitations involving Landau bands with Δ∣n∣=0Δ|n|=0 and with Δ∣n∣=±2Δ|n|=\pm2 that can be selected by controlling the angular momentum of the excitation laser and of the scattered light. The magneto-phonon effect involving the E2gE_{2g} optical phonon and KK-point inter Landau bands electronic excitations with Δ∣n∣=±1Δ|n|=\pm1 is revealed and analyzed within a model taking into account the full kzk_z dispersion. These polarization resolved results are explained in the frame of the Slonczewski-Weiss-McClure (SWM) model which directly allows to quantify the electron-hole asymmetry.

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