Electrodynamics of electron doped iron-pnictide superconductors: Normal state properties

preprint2010arXivOpen access

Abstract

The electrodynamic properties of Ba(Fe0.92_{0.92}Co0.08)2_{0.08})_2As2_{2} and Ba(Fe0.95_{0.95}Ni0.05)As_{0.05})_As_{2}singlecrystalshavebeeninvestigatedbyreflectivitymeasurementsinawidefrequencyrange.Inthemetallicstate,theopticalconductivityconsistsofabroadincoherentbackgroundandanarrowDrude−likecomponentwhichdeterminesthetransportproperties;onlythelattercontributionstronglydependsonthecompositionandtemperature.Thissubsystemrevealsa single crystals have been investigated by reflectivity measurements in a wide frequency range. In the metallic state, the optical conductivity consists of a broad incoherent background and a narrow Drude-like component which determines the transport properties; only the latter contribution strongly depends on the composition and temperature. This subsystem reveals a T^2behaviorinthedcresistivityandscatteringratedisclosingahiddenFermi−liquidbehaviorinthe122iron−pnictidefamily.AnextendedDrudeanalysisyieldsthefrequencydependenceoftheeffectivemass(with behavior in the dc resistivity and scattering rate disclosing a hidden Fermi-liquid behavior in the 122 iron-pnictide family. An extended Drude analysis yields the frequency dependence of the effective mass (with m^*/m_b\approx 5$ in the static limit) and scattering rate that does not disclose a simple power law. The spectral weight shifts to lower energies upon cooling; a significant fraction is not recovered within the infrared range of frequencies.

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