Drastic electronic structure reconstruction of Ca1−x_{1-x}Prx_xFe2_2As2_2 in the collapsed tetragonal phase

preprint2014arXivOpen access

Abstract

We report the electronic structure reconstruction of Ca1−x_{1-x}Prx_xFe2_2As2_2 (xx = 0.1 and 0.15) in the low temperature collapsed tetragonal (CT) phase observed by angle-resolved photoemission spectroscopy. Different from Ca(Fe1−x_{1-x}Rhx_x)2_2As2_2 and the annealed CaFe2_2As2_2 where all hole Fermi surfaces are absent in their CT phases, the cylindrical hole Fermi surface can still be observed in the CT phase of Ca1−x_{1-x}Prx_xFe2_2As2_2. Furthermore, we found at least three well separated electron-like bands around the zone corner in the CT phase of Ca1−x_{1-x}Prx_xFe2_2As2_2, which are more dispersive than the electron-like bands in the high temperature tetragonal phase. Based on these observations, we propose that the weakening of correlations (as indicated by the reduced effective mass), rather than the lack of Fermi surface nesting, might be responsible for the absence of magnetic ordering and superconductivity in the CT phase.

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