Disappearance of static magnetic order and evolution of spin fluctuations in Fe1+δ_{1+δ}Sex_{x}Te1−x_{1-x}

preprint2010arXivOpen access

Abstract

We report neutron scattering studies on static magnetic orders and spin excitations in the Fe-based chalcogenide system Fe1+δ_{1+δ}Sex_{x}Te1−x_{1-x} with different Fe and Se compositions. Short-range static magnetic order with the "bicollinear" spin configuration is found in all non-superconducting samples, with strong low-energy magnetic excitations near the (0.5,0)(0.5,0) in-plane wave-vector (using the two-Fe unit cell) for Se doping up to 45%. When the static order disappears and bulk superconductivity emerges, the spectral weight of the magnetic excitations shifts to the region of reciprocal space near the in-plane wave-vector (0.5,0.5)(0.5,0.5), corresponding to the "collinear" spin configuration. Our results suggest that spin fluctuations associated with the collinear magnetic structure appear to be universal in all Fe-based superconductors, and there is a strong correlation between superconductivity and the character of the magnetic order/fluctuations in

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