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Direct observation of moiré flat-band breakdown at the edge of magic-angle twisted bilayer graphene

Low-energy moiré flat bands in magic-angle twisted bilayer graphene (tBG) have demonstrated incredible potentials to exhibit rich exotic quantum phenomena. Theoretically, the moiré flat bands of tBG are based on the extended structures, i.e., the moiré patterns with periodic boundary conditions. However, a fundamental question of whether the flat bands can exist in the graphene moiré patterns with a reduced structure symmetry, such as sample edges, remains unanswered. Here, via scanning tunneling microscopy and spectroscopy, we study the local electronic properties of a magic-angle tBG near the sample terminated edge and report a direct observation of breakdown of the moiré flat bands. We show that the moiré electronic structures, including the low-energy flat bands, can sufficiently exist in a complete moiré spot, i.e., a moiré supercell, right at the edge even the translational symmetry of the moiré patterns is broken in one direction. However, the flat-band characteristic is obviously absent in the incomplete moiré spots that are partly terminated by the edge. Our results indicate that a whole moiré spot is sufficient and indispensable for the generation of the effective moiré flat bands in tBG.

preprint2022arXivOpen access
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Direct observation of moiré flat-band breakdown at the edge of magic-angle twisted bilayer graphene | BZPEER | BZPEER