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Determination of Gd concentration profile in UO2-Gd2O3 fuel pellets

A transversal mapping of the Gd concentration was measured in UO2-Gd2O3 nuclear fuel pellets by electron paramagnetic resonance spectroscopy (EPR). The quantification was made from the comparison with a Gd2O3 reference sample. The nominal concentration in the pellets is UO2: 7.5 % Gd2O3. A concentration gradient was found, which indicates that the Gd2O3 amount diminishes towards the edges of the pellets. The concentration varies from (9.3 +/- 0.5)% in the center to (5.8 +/- 0.3)% in one of the edges. The method was found to be particularly suitable for the precise mapping of the distribution of Gd3+ ions in the UO2 matrix.

preprint2014arXivOpen access
D. TobiaE. L. WinklerJ. MilanoA. ButeraR. KempfL. BianchiF. Kaufmann
cond-mat.mtrl-scinucl-ex
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Open access7 authors2 topics
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D. TobiaE. L. WinklerJ. MilanoA. ButeraR. KempfL. BianchiF. Kaufmann

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