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Crystallization of self-propelled hard-discs : a new scenario

We experimentally study the crystallization of a monolayer of vibrated discs with a built-in polar asymmetry, a model system of active liquids, and contrast it with that of vibrated isotropic discs. Increasing the packing fraction $ϕ$, the quasi-continuous crystallization reported for isotropic discs is replaced by a transition, or a crossover towards a "self-melting" crystal. Increasing the packing fraction from the liquid phase, clusters of dense hexagonally-ordered packed discs spontaneously form, melt, split and merge leading to a highly intermittent and heterogeneous dynamics. The resulting steady state cluster size distribution decreases monotonically. For packing fraction larger than $ϕ^*$, a few large clusters span the system size and the cluster size distribution becomes non monotonic, the transition being signed by a power-law. The system is however never dynamically arrested. The clusters permanently melt from place to place forming droplets of active liquid which rapidly propagate across the system. This state of affair remains up to the highest possible packing fraction questioning the stability of the crystal for active discs, unless at ordered close packing.

preprint2016arXivOpen access

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