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Arbitrary manipulation of nonlinear optical processes

Nonlinear optical processes are governed by the relative-phase relationships among the relevant electromagnetic fields in these processes. In this Letter, we describe the physics of arbitrary manipulation of nonlinear optical processes (AMNOP) by artificial control of relative phases. As a typical example, we show freely designable optical-frequency conversions to extreme spectral regions, mid-infrared and vacuum-ultraviolet, with near-unity quantum efficiencies. Furthermore, we show that such optical-frequency conversions can be realized by using a surprisingly simple technology where transparent plates are placed in a nonlinear optical medium and their positions and thicknesses are adjusted precisely. In a numerical experiment assuming practically applicable parameters in detail, we demonstrate a single-frequency tunable laser that covers the whole vacuum-ultraviolet spectral range of 120 to 200 nm.