Abstract

Neutral alkaline earth(-like) atoms have recently been employed in atomic arrays with individual readout, control, and high-fidelity Rydberg-mediated entanglement. This emerging platform offers a wide range of new quantum science applications that leverage the unique properties of such atoms: ultra-narrow optical "clock" transitions and isolated nuclear spins. Specifically, these properties offer an optical qubit ("o") as well as ground ("g") and metastable ("m") nuclear spin qubits, all within a single atom. We consider experimentally realistic control of this "omg" architecture and its coupling to Rydberg states for entanglement generation, focusing specifically on ytterbium-171 (171Yb^{171}\text{Yb}) with nuclear spin I=1/2I = 1/2. We analyze the SS-series Rydberg states of 171Yb^{171}\text{Yb}, described by the three spin-1/21/2 constituents (two electrons and the nucleus). We confirm that the F=3/2F = 3/2 manifold -- a unique spin configuration -- is well suited for entangling nuclear spin qubits. Further, we analyze the F=1/2F = 1/2 series -- described by two overlapping spin configurations -- using a multichannel quantum defect theory. We study the multilevel dynamics of the nuclear spin states when driving the clock or Rydberg transition with Rabi frequency Ωc=2π×200Ω_\text{c} = 2 π\times 200 kHz or ΩR=2π×6Ω_\text{R} = 2 π\times 6 MHz, respectively, finding that a modest magnetic field (≈200 G\approx200\,\text{G}) and feasible laser polarization intensity purity (≲0.99\lesssim0.99) are sufficient for gate fidelities exceeding 0.99.

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